Oscillations of partial oxidation of methane over H-ZSM-5 supported rhodium catalyst

Ying Liu

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Oscillations of partial oxidation of methane over H-ZSM-5 supported rhodium catalyst

Ying Liu * #

department of chemistry of Xiamen university

*Correspondence author

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Funding: none

Opened online: 4 April 2005

Accepted by: none

Citation: Ying Liu.Oscillations of partial oxidation of methane over H-ZSM-5 supported rhodium catalyst[OL]. [ 4 April 2005] http://en.paper.edu.cn/en_releasepaper/content/1797

The oscillatory behavior over the Rh/H-ZSM-5 catalyst was firstly reported at atmospheric pressure during the partial oxidation of methane. Temperature programmed techniques such as TPO and TPR were performed to look into the reaction mechanism. The results obtained from the experimental studies indicate that the synergism of the coke of some kind of stable form and the oxide which could be switching back and forth from the reduced state to the oxidized state is responsible for the oscillatory behavior seen in this system.

Keywords:methane partial oxidation, oscillations, Rh/H-ZSM-5 catalyst

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