Synthesis, photophysical and electrochemical properties of a D-π-A ensemble derived from porphyrazine and tetrathiafulvalene

Ruibin Hou; Han Qiu; Tie Chen; Bingzhu Yin

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Synthesis, photophysical and electrochemical properties of a D-π-A ensemble derived from porphyrazine and tetrathiafulvalene

Ruibin Hou 1,Han Qiu 1,Tie Chen 1,Bingzhu Yin 2 * #

1.Department of chemistry, Yanbian university

2.Key Laboratory of Natural Resources of Changbai Mountain & Functional Molecules (Yanbian University), Ministry of Education

*Correspondence author

#Submitted by

Subject:

Funding: 国家自然科学基金，教育部博士点基金（No.20662010,20060184001）

Opened online:10 June 2009

Accepted by: none

Citation: Ruibin Hou,Han Qiu,Tie Chen.Synthesis, photophysical and electrochemical properties of a D-π-A ensemble derived from porphyrazine and tetrathiafulvalene[OL]. [10 June 2009] http://en.paper.edu.cn/en_releasepaper/content/33006

Cis/trans 1,2-dicyanoethylenes bearing tetrathiafulvalene units linked by ethylenedithio spacer were prepared. The cis isomer was converted to eight tetrathiafulvalene unit substituted magnesium porphyrazine upon a metal-templated cyclotetramerization with magnesium propoxide in propanol. The dicyanoethylenes and target compound were characterized by EA, NMR, and MALDI-TOF mass and photophysical and Electrochemical propeties were discussed.

Keywords:tetrathiafulvalene;porphyrazine;dicyanoethylene;synthesis;electrochemistry

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