Brønsted Acid Catalyzed Benzylic C–H Bond Functionalization of Azaarenes: Nucleophilic Addition to Nitroso Compounds

Gao Xu; Yang Luo

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Brønsted Acid Catalyzed Benzylic C–H Bond Functionalization of Azaarenes: Nucleophilic Addition to Nitroso Compounds

Gao Xu,Yang Luo * #

College of Chemistry, Xiangtan University, Hunan

*Correspondence author

#Submitted by

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Funding: New Teachers’ Fund for Doctor Stations, Ministry of Education （No.20124301120007）

Opened online:30 June 2014

Accepted by: none

Citation: Gao Xu,Yang Luo.Brønsted Acid Catalyzed Benzylic C–H Bond Functionalization of Azaarenes: Nucleophilic Addition to Nitroso Compounds[OL]. [30 June 2014] http://en.paper.edu.cn/en_releasepaper/content/4602208

A practical Brønsted acid promoted benzylic C–H functionalization of 2-alkylazaarenes and nucleophilic addition to nitroso compounds was developed under mild conditions. Switched by Brønsted acids, this method can afford azaarene-2-aldimines, azaarene-2-carbaldehyde or azaarene-2-oximes selectively. No metal, base, oxidant or other additives were required.

Keywords:azaarene; Brønsted acid; nitroso compound

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